I've always thought "Schizophrenia" -- has both Thurston/Kim vocal parts and some very pretty/very atonal-dark passages, plus that great ending. Really, what's better?
Preferably a live version though...
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http://www.sonicyouth.com/mustang // original folk blues ... . . . . . . . . . . . . . . . . . . . . . . . . . . .i'm the boy that can enjoy invisibility. . . . . . . . . . . . . . . . . . . . . . . . .
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