Totally depends what type of music they already are into.
If they come from a punk rock background, maybe "World Looks Red".
If they smoke a lot of dope and like trippy stuff in general, probably "I Dreamed I Dream".
For a modern classical music fan (and I have met a couple who hadn't heard SY and were interested) probably something like "Anagrama" or "Free City Rhymes".
For an indie rock kid probably "Schizophrenia".
For a metalhead, definitely "Brother James".
That said, the first thing I heard was "She's in a Bad Mood" and it sure did the trick for me.
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