Tough call - it's a toss-up between S&E and Crooked Rain, Crooked Rain. I couldn't pick a favorite song.
And maybe I'm just bitter, but I'm not a fan of anything Malkmus did after Pavement, though I'm with Inhuman - I like him in the Silver Jews.
Of course I'd love Pavement to reform, but I doubt it's possible for them to recapture their original sound. Malkmus has changed his style too much post-Pavement to get that back.